IUPAC-NIST Solubility Database
NIST Standard Reference Database 106


Glass Ball as Bullet Solubility System: 2-Methyl-2-propanol with Benzene and Water

Components:
   (1) Water; H2O; [7732-18-5]  NIST Chemistry WebBook for detail
   (2) 2-Methyl-2-propanol (tert-butanol,tert-butyl alcohol); C4H10O; [75-65-0]  NIST Chemistry WebBook for detail
   (3) Benzene; C6H6; [71-43-2]  NIST Chemistry WebBook for detail

Evaluator:
   A. Skrzecz, Institute of Physical Chemistry, Polish Academy of Sciences, Warsaw, Poland (1997.05)

Critical Evaluation:

      A survey of reported compositions along the saturation curve (sat), and compositions of coexisting phases in equilibrium (eq.) for the system 2-methyl-2-propanol-benzene-water is given in Table 69.

Saturation curve
   The ternary system 2-methyl-2-propanol-benzene-water forms a miscibility gap of type 1. Only one binary system benzene-water forms a miscibility gap. These binary data were compiled and critically evaluated in a previously published SDS volume, Ref. 3. The recommended values of mutual solubility at 298 K are x'2=0.9970, x"2=0.000 409. The mutual solubility of benzene and water was also reported by Simonsen and Washburn,1 (x'2=0.9970, x"2=0.0003); these are consistent with the recommended values. Letcher et al.2 reported data only in graphical form. Therefore these data are not compiled. The plait point estimated by Letcher and Siswana4 was x1=0.16 and x2=0.02, while the maximum alcohol concentration on the binodal curve is x1=0.41. This point is consistent with the results of Simonsen and Washburn measurements, x1=0.38.1 The experimental tie lines at 298.2 K1 are presented in Fig. 36 together with the experimental points along the saturation curve.

Experimental Data:   (Notes on the Nomenclature)

TABLE 69. Summary of experimental data for the system 2-methyl-2-propanol-benzene-water
AuthorT/KDataTypeReference
Simonsen and Washburn, 1946298sat. (34), eq. (11)1
Letcher et al., 1990298sat. (13), eq. (4)2
View Figure 1 for this Evaluation

Notes:
Table 69  Number of experimental points in parentheses.

References: (Click a link to see its experimental data associated with the reference)

   1  Simonsen, D.R.; Washburn, E.R., J. Am. Chem. Soc. 68, 235 (1946).
   2  Letcher, T.M.; Sewry, J.; Radloff, S., S. Afr. J. Chem. 43, 56 (1990).
   3  Shaw, D.G., ed., Solubility Data Series, Vol. 37, Hydrocarbons with Water and Seawater, Part I: Hydrocarbons C5 to C7 (Pergamon, New York, 1989).
   4  Letcher, T.M.; Siswana, P.M., Fluid Phase Equilib. 74, 203 (1992).