IUPAC-NIST Solubility Database
NIST Standard Reference Database 106


Glass Ball as Bullet Solubility System: 2-Butanol with Cyclohexene and Water

Components:
   (1) Water; H2O; [7732-18-5]  NIST Chemistry WebBook for detail
   (2) 2-Butanol (sec-butanol, sec-butyl alcohol, (RS)-2-butanol, dl-2-butanol, DL-2-butanol); C4H10O; [78-92-2]  NIST Chemistry WebBook for detail
   (3) Cyclohexane; C6H12; [110-82-7]  NIST Chemistry WebBook for detail

Original Measurements:
   Letcher, T.M.; Siswana, P.; Radloff, S.E., S. Afr. J. Chem. 44, 118 (1991).

Variables:
   Temperature = 298 K

Prepared By:
   A. Skrzecz

Experimental Data:   (Notes on the Nomenclature)
  
Compositions along the saturation curve
t/°CT/KMass Fraction w1 (compiler) Mass Fraction w2 (compiler)Mole Fraction x1Mole Fraction x2
25.0298.20.0000.0000.0000.000
25.0298.20.1810.0000.0510.000
25.0298.20.6510.0000.3120.000
25.0298.20.6910.0130.3600.006
25.0298.20.7100.0270.3910.013
25.0298.20.7250.0700.4450.038
25.0298.20.6950.1740.5000.110
25.0298.20.6340.2730.5040.191
25.0298.20.5600.3740.4820.284
25.0298.20.4770.4770.4380.386
25.0298.20.3880.5810.3770.498
25.0298.20.2940.6870.3020.621
25.0298.20.1980.7920.2120.746
25.0298.20.1000.8970.1110.875
25.0298.20.0490.9490.0550.935
25.0298.20.00000.99980.0000.999
Compositions of coexisting phases
t/°CT/KMass Fraction w1 (compiler) Mass Fraction w2 (compiler)Mole Fraction x1Mole Fraction x2Comment(s)
25.0298.20.6510.0000.3120.000organic-rich phase
25.00298.20.7230.0740.4450.040organic-rich phase
25.00298.20.5940.3290.4950.241organic-rich phase
25.00298.20.4430.5170.4160.428organic-rich phase
25.00298.20.2710.7130.2800.650organic-rich phase
25.00298.20.1810.0000.0510.000water-rich phase
25.00298.20.1530.0000.0420.000water-rich phase
25.00298.20.1130.0000.0300.000water-rich phase
25.00298.20.0950.0000.0250.000water-rich phase
25.00298.20.0700.0000.0180.000water-rich phase
Method/Apparatus/Procedure:
   The points of the binodal curve were determined by the titration method, as described in Ref. 1. The formation of a cloudy mixture was observed visually on shaking after addition of a known mass of the third component; syringes were precisely weighed. Tie line compositions were determined by the refractive index method, Ref. 2, and a complementary method using the Karl Fischer titration, Ref. 3. Measurements were made at pressure of 94.7 kPa.

Source and Purity of Materials:
   (1) Merck; AR grade; dried by addition of anhydrous K2CO3, distilled; purity >99.9 mole % by glc.
   (2) BDH; Gold label grade; used as received; purity >99.9 mole % by glc.
   (3) Source not specified.

Estimated Errors:
   Solubility: Not reported.
   Temperature: Composition ±0.005 mole fraction (binodal curve), ±0.01 mole fraction (tie lines).

References:
   1 T. M. Letcher, S. Wootten, B. Shuttleworth, and C. Heyward, J. Chem. Thermodyn. 18, 1037 (1986).
   2 S. W. Briggs, and E. W. Comings, Ind. Eng. Chem. 35, 411 (1943).
   3 T. M. Letcher, P. Siswana, P. van der Watt, and S. Radloff, J. Chem. Thermodyn. 21, 1053 (1989).