IUPAC-NIST Solubility Database
NIST Standard Reference Database 106


Glass Ball as Bullet Solubility System: Carbon dioxide with Polyimide (PMDA-ODA) (Kapton H)

Components:
   (1) Carbon dioxide; CO2; [124-38-9]  NIST Chemistry WebBook for detail
   (2) Polyimide (PMDA-ODA) (Kapton H); ; [25036-53-7]  NIST Chemistry WebBook for detail

Original Measurements:
   K. Okamoto, K. Tanaka, O. Yokoshi and H. Kita, J. Polym. Sci., Part B: Polym. Phys. 27, 643 (1987).

Variables:
   Temperature = 323 K - 383 K
   Pressure = 0-2.7 MPa

Prepared By:
   S.M. Shishatski

Experimental Data:   (Subscripts 1,2,3, ..., in column headings refer to components 1,2,3, ...)
  
Dual mode sorption parameters for carbon dioxide in polyimide films
T/KHenry's law constant, K [cm3(STP)/cm3 atm]Langmuir's parameter, CH [cm3(STP) cm-3]Affinity Coefficient b [atm-1]Remark(s)
3230.90024.20.375Imidization at 473 K
3530.59917.70.206Imidization at 473 K
3830.42412.00.133Imidization at 473 K
3530.44410.60.226Imidization at 673 K
3230.63013.30.394Kapton-H
3530.4368.50.239Kapton-H
3830.2925.70.153Kapton-H
Method/Apparatus/Procedure:
   Pressure decay method was used for sorption measurements. The cell employed was similar to the one described in ref. (1).

Source and Purity of Materials:
   Polyimide was obtained by condensation of pyromellitic acid dianhidride and oxydiphenylenediamine with subsequent thermal imidization at 473 and 673 K. These samples and commercial polyimide Kapton H (Toray - DuPont Inc.) had the following densities: 1.405, 1.429, and 1.431 g/cm3, respectively. No information given on carbon dioxide purity.

Estimated Errors:


References:
   1 Koros, W.J.; Paul, D.R. J. Polym. Sci., Polym. Phys. Ed., 1976, 14, 1903.