IUPAC-NIST Solubility Database
NIST Standard Reference Database 106


Glass Ball as Bullet Solubility System: Nitromethane with Nitric acid and Water

Components:
   (1) Nitromethane; CH3NO2 ; [75-52-5]  NIST Chemistry WebBook for detail
   (2) Nitric acid; HNO3; [7697-37-2]  NIST Chemistry WebBook for detail
   (3) Water; H2O; [7732-18-5]  NIST Chemistry WebBook for detail

Original Measurements:
   Warner, R. K.; Aust. J. Appl. Sci. 4, 427-43 (1953).

Variables:
   Temperature = 293 K

Prepared By:
   V. P. Sazonov

Experimental Data:   (Notes on the Nomenclature)
  
Nitric acid  distribution between nitromethane-rich and water-rich phases
t/°CT/KMass Fraction w2Comment(s)
20.0293.20.140water-rich phase
20.0293.20.197water-rich phase
20.0293.20.258water-rich phase
20.0293.20.277water-rich phase
20.0293.20.286water-rich phase
20.0293.20.292water-rich phase
20.0293.20.286water-rich phase
20.0293.20.260water-rich phase
20.0293.20.195water-rich phase
20.0293.20.005nitromethane-rich phase
20.0293.20.016nitromethane-rich phase
20.0293.20.050nitromethane-rich phase
20.0293.20.075nitromethane-rich phase
20.0293.20.103nitromethane-rich phase
20.0293.20.136nitromethane-rich phase
20.0293.20.160nitromethane-rich phase
20.0293.20.177nitromethane-rich phase
20.0293.20.195 (a)nitromethane-rich phase
Notes:
   Table 1  a  System completely miscible.

Method/Apparatus/Procedure:
   The analytical method was used. The distribution of (2) between (1) and (3) was studied by preparing a mixture of aqueous nitric acid and nitromethane, such that after mixing the two phases were almost identical in composition. An extremely slow rate of phase separation of approximately equal volumes of each phase indicated this. Nitric acid (15 N) was added dropwise to the system and agitated until the system just became homogeneous. This condition was taken as the plait point and the termination of the distribution curve. The single-phase system was analyzed for nitric acid and the remaining points on the curve were obtained by adding successively increasing amounts of water to the system remaining after equilibration and analysis of the two phases from the previous determination. Nitric acid was determined in both phases by dilution of weighed aliquots with 100-150 mL of water and titration with 0.1 N potassium hydroxide to the methyl orange end point.

Source and Purity of Materials:
   (1) Source not specified; purity not specified; distilled.
   (2) Not specified.
   (3) Redistilled.

Estimated Errors:

   Temperature: control to ± 0.1 K.