IUPAC-NIST Solubility Database
NIST Standard Reference Database 106


Glass Ball as Bullet Solubility System: Ethanol with Benzene and Water

Components:
   (1) Water; H2O; [7732-18-5]  NIST Chemistry WebBook for detail
   (2) Benzene; C6H6; [71-43-2]  NIST Chemistry WebBook for detail
   (3) Ethanol (ethyl alcohol); C2H6O; [64-17-5]  NIST Chemistry WebBook for detail

Original Measurements:
   Washburn, E.R., Hnizda, V.; Vold, R., J. Am. Chem. Soc. 53, 3237 (1931).

Variables:
   Temperature = 298 K

Prepared By:
   A. Skrzecz

Experimental Data:   (Notes on the Nomenclature)
  
Compositions along the saturation curve
t/°CT/KMass Fraction w1Mass Fraction w2Mole Fraction x1 (compiler)Mole Fraction x2 (compiler)
24.5297.70.0820.9110.12870.8432
24.5297.70.1000.8900.15370.8070
24.5297.70.1290.8570.19250.7541
24.5297.70.1790.7950.25060.6564
24.5297.70.2530.7020.32350.5294
24.5297.70.2910.6460.34930.4571
24.5297.70.3430.5700.38040.3728
24.5297.70.4160.4620.41580.2723
24.5297.70.4480.3980.41610.2180
24.5297.70.5040.2790.41190.1345
24.5297.70.5180.2300.39910.1045
24.5297.70.5120.1140.33340.0438
24.5297.70.4660.0510.26920.0174
24.5297.70.3740.0210.19340.0064
24.5297.70.2990.00830.14410.0024
24.5297.70.2580.00570.12030.0016
Distribution of ethanol in ethanol-benzene-water system
t/°CT/KMass Fraction w1Comment(s)
25.0298.20.007hydrocarbon-rich phase
25.0298.20.012hydrocarbon-rich phase
25.0298.20.016hydrocarbon-rich phase
25.0298.20.024hydrocarbon-rich phase
25.0298.20.039hydrocarbon-rich phase
25.0298.20.054hydrocarbon-rich phase
25.0298.20.070hydrocarbon-rich phase
25.0298.20.084hydrocarbon-rich phase
25.0298.20.098hydrocarbon-rich phase
25.0298.20.025water-rich phase
25.0298.20.106water-rich phase
25.0298.20.164water-rich phase
25.0298.20.243water-rich phase
25.0298.20.318water-rich phase
25.0298.20.370water-rich phase
25.0298.20.405water-rich phase
25.0298.20.443water-rich phase
25.0298.20.573water-rich phase
Method/Apparatus/Procedure:
   The titration method was used. Binary alcohol-benzene mixtures of known composition, prepared from calibrated pipettes in 125 mL glass-stoppered bottles, were mixed, and titrated with water to a permanent cloudiness at room temperature (24.5°C). The amount of water was 0.66-5.77 mL (added from a 10 mL burette graduated to 0.01 mL) and 17.1-112.7 mL (added from a calibrated 50 mL burette). The refractive indexes of mixtures were measured at 25.°C by Abbe  refractometer and used to construct the plot of refractive index against composition which was further used to find compositions of equilibrium phases. Phase equilibrium data were reported in incomplete form. The mixtures of 25.0 mL of benzene and 25.0 mL of water were shaken and then suspended in the constant temperature bath to reach equilibrium. When the phases were  transparent, refractive indexes of each layer were measured and composition of the phases were calculated.

Source and Purity of Materials:
   (1) Standard commercial grade of absolute alcohol; dried with CaCO and Ca until density measurements showed it to be better than 99.3%.
   (2) Mallinckrodt, reagent quality; dried with Na, distilled.
   (3) Redistilled from KMnO4.

Estimated Errors:
   Solubility: Not reported.
   Temperature: Temp. ±0.1°C.